Journalartikel

Separation of atomic and molecular ions by ion mobility with an RF carpet


AutorenlisteMiskun, Ivan; Dickel, Timo; San Andres, Samuel Ayet; Bergmann, Julian; Constantin, Paul; Ebert, Jens; Geissel, Hans; Greiner, Florian; Haettner, Emma; Hornung, Christine; Lippert, Wayne; Mardor, Israel; Moore, Iain; Plass, Wolfgang R.; Purushothaman, Sivaji; Rink, Ann-Kathrin; Reiter, Moritz P.; Scheidenberger, Christoph; Weick, Helmut

Jahr der Veröffentlichung2021

ZeitschriftInternational Journal of Mass Spectrometry

Bandnummer459

ISSN1387-3806

eISSN1873-2798

Open Access StatusHybrid

DOI Linkhttps://doi.org/10.1016/j.ijms.2020.116450

VerlagElsevier


Abstract
Gas-filled stopping cells are used at accelerator laboratories for the thermalization of high-energy radioactive ion beams. Common challenges of many stopping cells are a high molecular background of extracted ions and limitations of extraction efficiency due to space-charge effects. At the FRS Ion Catcher at GSI, a new technique for removal of ionized molecules prior to their extraction out of the stopping cell has been developed. This technique utilizes the RF carpet for the separation of atomic ions from molecular contaminant ions through their difference in ion mobility. Results from the successful implementation and test during an experiment with a 600 MeV/u Xe-124 primary beam are presented. Suppression of molecular contaminants by three orders of magnitude has been demonstrated. Essentially background-free measurement conditions with less than 1 % of background events within a mass-to charge range of 25 u/e have been achieved. The technique can also be used to reduce the space charge effects at the extraction nozzle and in the downstream beamline, thus ensuring high efficiency of ion transport and highly-accurate measurements under space-charge-free conditions. (C) 2020 The Author(s). Published by Elsevier B.V.



Zitierstile

Harvard-ZitierstilMiskun, I., Dickel, T., San Andres, S., Bergmann, J., Constantin, P., Ebert, J., et al. (2021) Separation of atomic and molecular ions by ion mobility with an RF carpet, International Journal of Mass Spectrometry, 459, Article 116450. https://doi.org/10.1016/j.ijms.2020.116450

APA-ZitierstilMiskun, I., Dickel, T., San Andres, S., Bergmann, J., Constantin, P., Ebert, J., Geissel, H., Greiner, F., Haettner, E., Hornung, C., Lippert, W., Mardor, I., Moore, I., Plass, W., Purushothaman, S., Rink, A., Reiter, M., Scheidenberger, C., & Weick, H. (2021). Separation of atomic and molecular ions by ion mobility with an RF carpet. International Journal of Mass Spectrometry. 459, Article 116450. https://doi.org/10.1016/j.ijms.2020.116450



Schlagwörter


Beam purificationGAS CELLLow-energy RIBMolecular contaminationSpace charge

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